Three Apple Varieties Show Differences in Organic Composition when Reducing Sugars, Pigments and Enzymes are Tested.
By: Leslie Madden, Michael Rak Elizabeth Brown

ABSTRACT:
Three apple varieties were investigated in order to determine the differences in their organic make-up. In order to parameterize this make-up, we chose to characterize the reducing sugar content, the pigment content, and the enzyme activity. In quantifying the reducing sugar content, Benedict’s test for reducing sugars was run and the resulting solutions were placed in a spectrophotometer to quantify the sugar content. To characterize the pigments in the skins of our apple varieties, paper chromatography was used. The absorption spectrum was then taken to clearly represent the differences in the pigments. The next test was done to display the activity of polyphenol oxidase (PPO) when it was placed into different environments and the difference between the three apple types regarding the activity of the PPO in each variety. Our experiments provided evidence that there were different quantities of Free Ketoses and Aldoses in the three apple varieties. There is Evidence that the Red Delicious and Granny Smiths had few similar pigments, while Fuji apples had some pigments that were the same as Red Delicious and some that were similar to the Granny Smith apples. We found that PPO works best when in a basic environment and that the Granny Smith apples tend to contain the most PPO, whose content is much greater than both the Red Delicious and the Fuji varieties. The evidence contained herein supports the hypothesis, that, although these three fruits tested are all apples, on the molecular level they are not identical.

DISCUSSION:
The three different apples, from the everyday human perspective, appear quite similar, but as we have found out are actually quite different. In the first experiment, tests were run to qualitatively determine the presence of different types of carbohydrates or sugars. These tests yielded similar results for all the apples because all three formed a precipitate when the Benedict’s test was run. This verifies that all three apples have free Aldhyde and Ketone groups present. An inherent flaw of the Benedict’s experiment was that there were no quantitative results. This afforded us no ability to determine which apples had high or low sugar levels. We suspected that there was a difference, due to the fact that the apples have different degrees of sweetness and bitterness on the palate. Dr. Luckie recommended that we run our final solution after the Benedict’s test through a spectrophotometer to solve this problem. In order for the absorbance spectrum to read our results we had to dilute the solutions after the Benedict’s test. It was hard to make sure that all of the precipitate was evenly distributed throughout the solution. This was also a problem when placing the cuvettes in the spectrophotometer because the precipitate tended to settle quickly. Since this occurred for all of the trials we feel that this has very little effect on our results. A second inherent flaw of this first experiment is that the apples used could be at different points of ripeness, which would cause different concentrations of different sugars as well. A way to minimize this is to pick the apples by hand on the day that the experiment is occurring. Unfortunately this was too difficult for us to do with the resources at hand.

When running the spectrophotometer we tested for the % Transmittance. The higher the % transmittance the more light is allowed to travel through. This means that there is less precipitate in solution. We originally predicted that the Granny Smith, Fuji, and then Red Delicious would have the highest to lowest % transmittance. We found that Red Delicious had the highest % transmittance, the Fuji apples had the next and the Granny Smiths had the lowest.

Experiment 2 was a pigment comparison of the three types of apples. This experiment did not follow our predicted results; we felt that the Fuji would have pigments that were closer to the Red Delicious since they are closer in lineage than they are to Granny Smith apples. We ran two trials for each apple variety and did not see variation between the trials for each variety. With the Granny Smith Apples we found that there were at least three different pigments. For the Fuji apples we found that there was only one pigment present which seemed to match with the last line of pigment for the Granny Smith. Unfortunately for the Red Delicious apple we only got very faint to no results. We feel that the reason this occurred is because we were not able to get a solution of pure pigment for the Red Delicious to place on the filter paper. (Figure 15) If what we thought was pigment but instead was the fruit of the apple then there would be little to no pigment since the fruit of the apple is white. If we were to redo this portion of our experiment it would be helpful to find a way to minimize the amount of fruit left on the apple peel. We can conclude from the experiment that even though the Fuji and Granny Smith apples are not genealogically related, they seem to share at least one pigment. This pigment may be a pigment found in all apples or more broadly in plants, but more research needs to be done to confirm this.

In experiment 3, we attempted to characterize the nature and amount of PPO in each of the three varieties of apples. In this experiment, we observed that the Red Delicious browned the fastest, followed by the Granny Smith, and the Fuji’s. This led us to believe that the Red Delicious had the most PPO. When testing to see if the apple pieces were affected by different pH levels we obtained some interesting results. The lemon juice and the Fruit-Fresh kept the apple from turning brown for about the same length of time, although, the Fresh-fruit worked a little bit better. We feel that the reason for this difference is because of the dextrose that is present in Fruit Fresh. The basic solution that consisted of baking soda caused the apple to brown the fastest. We feel this was because the acid irreversibly denatured the enzyme where as the base catalyzes the PPO enzyme reaction. From this experiment we were able to conclude that the best way to prevent fruit from browning would be to coat it ideally with the product Fresh-Fruit or for a cheaper alternative to use lemon juice. It would be interesting to test other edible household products to see if they have any effect on the PPO reactions.

With all of the evidence at hand, we conclude that although all three selections are all apples, there are a few things that are chemically different. This provides quite an interesting outcome and platform for potential future research within the realm of the apple.

 

Figure 16: These are the results of the first part of the PPO testing after 30 minutes. They were cut and treated with catechol. The resulting brown color is from the PPO in the apples reducing the catechol. From the left upper corner it is Granny Smith, Red Delicious and Fuji apple.

 

REFERENCES:
Dennis, Frank. Apple Varieties, yesterday, today and tomorrow: East Lansing, MI, Michigan State University, 1996.

Marshall, Brian. “Question of the Day: Why do apples and potatoes turn brown?”
How Stuff Works (1999-2002): accessed 8-29-02
< http://www.howstuffworks.com/question168.htm >

“Varieties” Washington Apples (2002): accessed 8-29-02
< http://www.bestapples.com/apple-info/varieties/ >

“Granny Smith Apples” Fruit from Washington (7-22-02): accessed 8-29-02
< http://www.fruitfromwashington.com/Varieties/grannysmith.htm